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Delivering audible content to a targeted listener without disturbing others is paramount in audio engineering. However, achieving this goal has long been challenging due to the diffraction of low-frequency (long-wavelength) audio waves in linear acoustics. Here, we introduce an approach for creating remote audio spots, dubbed audible enclaves, by harnessing the local nonlinear interaction of two self-bending ultrasonic beams with distinct spectra. The self-bending ultrasonic beams created by acoustic metasurfaces, though inaudible, can bypass obstacles such as human heads. At their intersection behind obstacles, highly localized audible enclaves are formed due to the local nonlinear interactions. Additionally, we demonstrate the ultrabroadband capabilities of our metasurface-based implementation both numerically and experimentally, spanning from 125 Hz to 4 kHz (6 octave bands), covering the majority of the audible frequency range. The practicality of our proposed technique is underscored by its compact implementation size (0.16 m, equivalent to 0.06 wavelengths at 125 Hz), as well as its robust performance under wideband transient audio signal excitation and in a common room with reverberations. Our proposed audible enclaves hold significant potential for various applications in advanced audio engineering, including private speech communications, immersive spatial audio reproduction, and high-resolution sound/quiet zone control. 

Understanding and exploiting material flexibility through phenomena such as the bending and twisting of molecular crystals has been a subject of increased interest owing to the number of applications that benefit from these properties, such as optoelectronics, mechanophotonics, soft robotics, and smart sensors. Here, we report the growth of spontaneously bent and twisted ammonium urate crystals induced by the keto–enol tautomerism of the urate molecule. The major tautomer is native to biogenic crystals, whereas the minor tautomer functions as an effective crystal growth modifier to induce naturally bent and twisted ammonium urate crystals. We show that the degree of curvature can be tailored based on the judicious selection of growth conditions. A combination of state-of-the-art microscopy and spectroscopy techniques are used to characterize the origin of bending. Spatially resolved nano-electron diffraction and high-resolution electron microscopy of naturally bent crystals show nearly single crystallinity with local lattice deformations generated by a combination of screw and edge dislocations. These observations are consistent with photoinduced force microscopy and contact resonance atomic force microscopy, which confirmed spatially resolved changes in the intermolecular interactions and the mechanical properties throughout the cross-sectional and axial regions of bent crystals. A mechanism of bending involving the generation of regionally specific dislocations is proposed as an alternative to more commonly reported models. These findings highlight a unique characteristic of tautomeric crystals that may have broader implications for other biogenic materials. 

Abstract Acoustic metasurfaces are at the frontier of acoustic functional material research owing to their advanced capabilities of wave manipulation at an acoustically vanishing size. Despite significant progress in the last decade, conventional acoustic metasurfaces are still fundamentally limited by their underlying physics and design principles. First, conventional metasurfaces assume that unit cells are decoupled and therefore treat them individually during the design process. Owing to diffraction, however, the non-locality of the wave field could strongly affect the efficiency and even alter the behavior of acoustic metasurfaces. Additionally, conventional acoustic metasurfaces operate by modulating the phase and are typically treated as lossless systems. Due to the narrow regions in acoustic metasurfaces’ subwavelength unit cells, however, losses are naturally present and could compromise the performance of acoustic metasurfaces. While the conventional wisdom is to minimize these effects, a counter-intuitive way of thinking has emerged, which is to harness the non-locality as well as loss for enhanced acoustic metasurface functionality. This has led to a new generation of acoustic metasurface design paradigm that is empowered by non-locality and non-Hermicity, providing new routes for controlling sound using the acoustic version of 2D materials. This review details the progress of non-local and non-Hermitian acoustic metasurfaces, providing an overview of the recent acoustic metasurface designs and discussing the critical role of non-locality and loss in acoustic metasurfaces. We further outline the synergy between non-locality and non-Hermiticity, and delineate the potential of using non-local and non-Hermitian acoustic metasurfaces as a new platform for investigating exceptional points, the hallmark of non-Hermitian physics. Finally, the current challenges and future outlook for this burgeoning field are discussed. 

There is a trade-off between the sparseness of an absorber array and its sound absorption imposed by wave physics. Here, near-perfect absorption (99% absorption) is demonstrated when the spatial period of monopole-dipole resonators is close to one working wavelength (95% of the wavelength). The condition for perfect absorption is to render degenerate monopole-dipole resonators critically coupled. Frequency domain simulations, eigenfrequency simulations, and the coupled mode theory are utilized to demonstrate the acoustic performances and the underlying physics. The sparse-resonator-based sound absorber could greatly benefit noise control with air flow and this study could also have implications for electromagnetic wave absorbers. 

Architected metamaterials have emerged as a central topic in materials science and mechanics, thanks to the rapid development of additive manufacturing techniques, which have enabled artificial materials with outstanding mechanical properties. This Letter seeks to investigate the elastodynamic behavior of octet truss lattices as an important type of architected metamaterials for high effective strength and vibration shielding. We design, fabricate, and experimentally characterize three types of octet truss structures, including two homogenous structures with either thin or thick struts and one hybrid structure with alternating strut thickness. High elastic wave transmission rate is observed for the lattice with thick struts, while strong vibration mitigation is captured from the homogenous octet truss structure with thin struts as well as the hybrid octet truss lattice, though the underlying mechanisms for attenuation are fundamentally different (viscoelasticity induced dampening vs bandgaps). Compressional tests are also conducted to evaluate the effective stiffness of the three lattices. This study could open an avenue toward multifunctional architected metamaterials for vibration shielding with high mechanical strength.